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Global atmospheric particle formation from CERN CLOUD measurements

Identifieur interne : 000057 ( Main/Exploration ); précédent : 000056; suivant : 000058

Global atmospheric particle formation from CERN CLOUD measurements

Auteurs : Eimear M. Dunne [Royaume-Uni] ; Hamish Gordon [Suisse] ; Andreas Kürten [Allemagne] ; Joao Almeida [Suisse] ; Jonathan Duplissy [Finlande] ; Christina Williamson [Allemagne] ; Ismael K. Ortega Colomer [France] ; Kirsty J. Pringle [Royaume-Uni] ; Alexey Adamov [Finlande] ; Urs Baltensperger [Suisse] ; Peter Barmet [Suisse] ; François Benduhn [Allemagne] ; Federico Bianchi [Finlande] ; Martin Breitenlechner [France] ; Anthony Clarke [États-Unis] ; Joachim Curtius [Allemagne] ; Josef Dommen [Suisse] ; Neil M. Donahue [Finlande] ; Sébastian Ehrhart [Suisse] ; Rchard C. Flagan [États-Unis] ; Alessandro Franchin [Finlande] ; Roberto Guida [Royaume-Uni] ; Jani Hakala [Finlande] ; A. Hansel [Finlande] ; Martin Heinritzi [Allemagne] ; Tuija Jokinen [Finlande] ; Juha Kangasluoma [Finlande] ; Jasper Kirkby [Suisse] ; Markku Kulmala [Finlande] ; Agnieszka Kupe [Autriche] ; Michael J. Lawler [Finlande] ; Katrianne Lehtipalo [Finlande] ; Vladimir Makhmutov [Russie] ; Graham Mann [Royaume-Uni] ; Serge Mathot [Suisse] ; Joonas Merikanto [Finlande] ; Pasi Miettinen [Finlande] ; Athanasios Nenes [Grèce] ; Antti Onnela [Suisse] ; Alexandru Rap [Royaume-Uni] ; Carly L. S. Reddington [Royaume-Uni] ; Francesco Riccobono [Suisse] ; Nigel A. D. Richard [Royaume-Uni] ; Matti P. Rissanen [Finlande] ; Linda Rondo [Allemagne] ; Nina Sarnela [Finlande] ; Siegfried Schobesberger [Finlande] ; Kamalika Sengupta [Royaume-Uni] ; Mario Simon [Allemagne] ; Mikko Sipil [Finlande] ; James N. Smith [Finlande] ; Yuri Stozkhov [Russie] ; Antonio Tomé [Portugal] ; Jasmin Tröstl [Suisse] ; Paul E. Wagner [Autriche] ; Daniela Wimmer [Allemagne] ; Paul M. Winkler [Autriche] ; Douglas R. Worsnop [États-Unis] ; Kenneth S. Carslaw [Royaume-Uni]

Source :

RBID : Hal:hal-01397769

English descriptors

Abstract

Fundamental questions remain about the origin of newly formed atmospheric aerosol particles becausedata from laboratory measurements have been insufficient to build global models. In contrast, gas-phasechemistry models have been based on laboratory kinetics measurements for decades. Here we build aglobal model of aerosol formation using extensive laboratory-measured nucleation rates involving sulfuricacid, ammonia, ions and organic compounds. The simulations and a comparison with atmosphericobservations show that nearly all nucleation throughout the present-day atmosphere involves ammonia orbiogenic organic compounds in addition to sulfuric acid. A significant fraction of nucleation involves ions,but the relatively weak dependence on ion concentrations indicates that for the processes studiedvariations in cosmic ray intensity do not significantly affect climate via nucleation in the present-dayatmosphere.

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<orgName>Solar and Cosmic Ray Research Laboratory [Moscow]</orgName>
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<orgName>P. N. Lebedev Physical Institute of the Russian Academy of Sciences</orgName>
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<addrLine>Leninsky prospekt., 53, Moscow 117924</addrLine>
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</address>
<ref type="url">http://www.lebedev.ru/</ref>
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<orgName>Russian Academy of Sciences [Moscow]</orgName>
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<addrLine>Leninsky Ave, 14, Moscow, Russie, 119991</addrLine>
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<ref type="url">http://www.ras.ru/en/index.aspx</ref>
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<country>Russie</country>
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</author>
<author>
<name sortKey="Tome, Antonio" sort="Tome, Antonio" uniqKey="Tome A" first="Antonio" last="Tomé">Antonio Tomé</name>
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<orgName>CENTRA-SIM</orgName>
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<orgName>IDL-Faculdade de Ciencias da Universidade de Lisboa</orgName>
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<address>
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</address>
</desc>
</org>
</tutelle>
</tutelles>
</hal:affiliation>
<country>Portugal</country>
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</author>
<author>
<name sortKey="Trostl, Jasmin" sort="Trostl, Jasmin" uniqKey="Trostl J" first="Jasmin" last="Tröstl">Jasmin Tröstl</name>
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<hal:affiliation type="laboratory" xml:id="struct-60801" status="INCOMING">
<orgName>Laboratory of Atmospheric Chemistry</orgName>
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<orgName>Laboratory of Atmospheric Chemistry</orgName>
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</desc>
</org>
</tutelle>
</tutelles>
</hal:affiliation>
<country>Suisse</country>
</affiliation>
</author>
<author>
<name sortKey="Wagner, Paul E" sort="Wagner, Paul E" uniqKey="Wagner P" first="Paul E." last="Wagner">Paul E. Wagner</name>
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<hal:affiliation type="laboratory" xml:id="struct-109401" status="VALID">
<orgName>Faculty of Physics [Vienna]</orgName>
<desc>
<address>
<addrLine>Boltzmanngasse 5, 1090 Wien</addrLine>
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<ref type="url">http://physik.univie.ac.at/</ref>
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<orgName>Universität Wien</orgName>
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<addrLine>Universitätsring 1, 1010 Wien</addrLine>
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<ref type="url">https://www.univie.ac.at/</ref>
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</org>
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</tutelles>
</hal:affiliation>
<country>Autriche</country>
</affiliation>
</author>
<author>
<name sortKey="Wimmer, Daniela" sort="Wimmer, Daniela" uniqKey="Wimmer D" first="Daniela" last="Wimmer">Daniela Wimmer</name>
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<orgName>Institute for Atmospheric and Environmental Sciences [Frankfurt/Main]</orgName>
<orgName type="acronym">IAU</orgName>
<desc>
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<addrLine>Altenhöferallee 1, 60438 Frankfurt/Main</addrLine>
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</address>
<ref type="url">http://www.goethe-university-frankfurt.de/45678073/IAU</ref>
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<orgName>Goethe-University Frankfurt am Main</orgName>
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<address>
<addrLine>Theodor-W.-Adorno-Platz 1 , 60323 Frankfurt am Main</addrLine>
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</address>
<ref type="url">http://www.goethe-university-frankfurt.de/en?</ref>
</desc>
</org>
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</tutelles>
</hal:affiliation>
<country>Allemagne</country>
</affiliation>
</author>
<author>
<name sortKey="Winkler, Paul M" sort="Winkler, Paul M" uniqKey="Winkler P" first="Paul M." last="Winkler">Paul M. Winkler</name>
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<hal:affiliation type="laboratory" xml:id="struct-109401" status="VALID">
<orgName>Faculty of Physics [Vienna]</orgName>
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<address>
<addrLine>Boltzmanngasse 5, 1090 Wien</addrLine>
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</address>
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</desc>
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<orgName>Universität Wien</orgName>
<desc>
<address>
<addrLine>Universitätsring 1, 1010 Wien</addrLine>
<country key="AT"></country>
</address>
<ref type="url">https://www.univie.ac.at/</ref>
</desc>
</org>
</tutelle>
</tutelles>
</hal:affiliation>
<country>Autriche</country>
</affiliation>
</author>
<author>
<name sortKey="Worsnop, Douglas R" sort="Worsnop, Douglas R" uniqKey="Worsnop D" first="Douglas R." last="Worsnop">Douglas R. Worsnop</name>
<affiliation wicri:level="1">
<hal:affiliation type="institution" xml:id="struct-314746" status="VALID">
<orgName>Aerodyne Research Inc.</orgName>
<desc>
<address>
<addrLine>45 Manning Rd, Billerica, MA 01821</addrLine>
<country key="US"></country>
</address>
<ref type="url">http://www.aerodyne.com</ref>
</desc>
</hal:affiliation>
<country>États-Unis</country>
</affiliation>
</author>
<author>
<name sortKey="Carslaw, Kenneth S" sort="Carslaw, Kenneth S" uniqKey="Carslaw K" first="Kenneth S." last="Carslaw">Kenneth S. Carslaw</name>
<affiliation wicri:level="1">
<hal:affiliation type="institution" xml:id="struct-123346" status="VALID">
<orgName>University of Leeds</orgName>
<desc>
<address>
<addrLine>Woodhouse Lane, Leeds LS2 9JT</addrLine>
<country key="GB"></country>
</address>
<ref type="url">http://www.leeds.ac.uk/</ref>
</desc>
</hal:affiliation>
<country>Royaume-Uni</country>
</affiliation>
</author>
</analytic>
<series>
<title level="j">Science</title>
<idno type="ISSN">0036-8075</idno>
<imprint>
<date type="datePub">2016-10-27</date>
</imprint>
</series>
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</sourceDesc>
</fileDesc>
<profileDesc>
<textClass>
<keywords scheme="mix" xml:lang="en">
<term>CLIMATE</term>
<term>GLOBAL MODELING</term>
<term>NUCLEATION</term>
</keywords>
</textClass>
</profileDesc>
</teiHeader>
<front>
<div type="abstract" xml:lang="en">Fundamental questions remain about the origin of newly formed atmospheric aerosol particles becausedata from laboratory measurements have been insufficient to build global models. In contrast, gas-phasechemistry models have been based on laboratory kinetics measurements for decades. Here we build aglobal model of aerosol formation using extensive laboratory-measured nucleation rates involving sulfuricacid, ammonia, ions and organic compounds. The simulations and a comparison with atmosphericobservations show that nearly all nucleation throughout the present-day atmosphere involves ammonia orbiogenic organic compounds in addition to sulfuric acid. A significant fraction of nucleation involves ions,but the relatively weak dependence on ion concentrations indicates that for the processes studiedvariations in cosmic ray intensity do not significantly affect climate via nucleation in the present-dayatmosphere.</div>
</front>
</TEI>
<affiliations>
<list>
<country>
<li>Allemagne</li>
<li>Autriche</li>
<li>Finlande</li>
<li>France</li>
<li>Grèce</li>
<li>Portugal</li>
<li>Royaume-Uni</li>
<li>Russie</li>
<li>Suisse</li>
<li>États-Unis</li>
</country>
</list>
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<noRegion>
<name sortKey="Dunne, Eimear M" sort="Dunne, Eimear M" uniqKey="Dunne E" first="Eimear M." last="Dunne">Eimear M. Dunne</name>
</noRegion>
<name sortKey="Carslaw, Kenneth S" sort="Carslaw, Kenneth S" uniqKey="Carslaw K" first="Kenneth S." last="Carslaw">Kenneth S. Carslaw</name>
<name sortKey="Guida, Roberto" sort="Guida, Roberto" uniqKey="Guida R" first="Roberto" last="Guida">Roberto Guida</name>
<name sortKey="Mann, Graham" sort="Mann, Graham" uniqKey="Mann G" first="Graham" last="Mann">Graham Mann</name>
<name sortKey="Pringle, Kirsty J" sort="Pringle, Kirsty J" uniqKey="Pringle K" first="Kirsty J." last="Pringle">Kirsty J. Pringle</name>
<name sortKey="Rap, Alexandru" sort="Rap, Alexandru" uniqKey="Rap A" first="Alexandru" last="Rap">Alexandru Rap</name>
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<name sortKey="Winkler, Paul M" sort="Winkler, Paul M" uniqKey="Winkler P" first="Paul M." last="Winkler">Paul M. Winkler</name>
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